Permeable Reactive Barriers (Proceedings of the International Symposium held at Belfast, Northern Ireland, March 2004). IAHS Publ. 298, 2005, 117-122.


Remediation of acidic colliery spoil leachate in a hybrid passive treatment system comprising a permeable reactive barrier, ponds and a reedbed (Shilbottle, Northumberland, UK)

PAUL L. YOUNGER & MAHMOUD MOUSTAFA

School of Civil Engineering and Geosciences, Drummond Building, University of Newcastle, Newcastle upon Tyne NE1 7RU, UK

paul.younger@ncl.ac.uk

Abstract Highly acidic spoil leachates at the former Shilbottle Grange Colliery site (Northumberland, UK) have been constrained to flow through a permeable reactive barrier (PRB) containing a mixture of limestone gravel, horse manure and composted green waste. Leachates leave the PRB through a seepage face, draining into ponds and a reedbed. Iron concentrations decrease across the system from >800 mg l-1 to ~ 10 mg l-1. Iron loading reduction is about 98%. While pH rises from 4 to 6 in the PRB, subsequent precipitation of metals as hydroxides and hydroxysulphates leads to the apparent paradox of simultaneous decreases in both total acidity and pH. The PRB removes about 30% of the sulphate (by reductive precipitation of metal sulphides), while the lagoons and reed bed together remove another 20% (as hydroxy-sulphate precipitates). The system as a whole reduces the sulphate content of the raw water by 50%.

Key words acidic mine drainage; geochemistry; groundwater; mining; permeable reactive barrier; pollution; remediation; treatment; spoil; UK; wetlands